You can't ungroup them, but you can de-select the autolayout so that you can
move individual boxes around. To do so, click on the org chart, then right
click on one of the individual boxes, then click Layout > Autolayout.
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But also, if you really need to ungroup the org chart for some reason,
select it and copy it, then choose Edit|Paste Special|Picture-Enhanced
Metafile (EMF). Then select the EMF and ungroup it twice.